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Self-sealing mafic sills for carbon and hydrogen storage Available to Purchase
Abstract Tabular igneous intrusions (sills) are common features in sedimentary basins and have the potential to be useful seals for fluids (e.g. CO 2 or H 2 ) in geological storage scenarios, and may be important as the need for geological carbon sequestration and alternative fuel storage increases. This is advantageous in regions without ready access to large-volume reservoirs in depleted hydrocarbon plays and saline aquifers, such as the northeastern USA. Moreover, geological H 2 storage requires more demanding conditions than those typically associated with oil and gas. An enhanced seal will have the properties of a traditional seal – competent, low permeability and laterally extensive – with the addition of being able to self-seal pre-existing and induced fractures. Self-sealing will occur along fluid pathways like fractures where CO 2 , water and minerals like plagioclase, olivine and pyroxene react together. Dolerite sills from the Gettysburg Basin, Pennsylvania, have remarkably low permeability and homogeneous compositions that include minerals that will readily react with CO 2 dissolved in water. Here, we characterize the physical properties and chemical gradients within several mafic sills cored in five boreholes. In addition, preliminary CO 2 -reaction experiments on dolerite samples demonstrated rapid carbonate mineralization.
The structure, fabrics and AMS of the Slieve Gullion ring-complex, Northern Ireland: testing the ring-dyke emplacement model Available to Purchase
Abstract A structural investigation of the Slieve Gullion ring-complex, part of the approximately 56 Ma Slieve Gullion Igneous Centre, County Armagh, Northern Ireland was carried out with a view to testing the ring-dyke emplacement mechanism. This investigation involved the detailed examination and mapping of critical field relationships and the measurement of visible and magnetic fabrics, within the porphyritic rhyolite (felsite) and the porphyritic granite (granophyre) parts of the ring-complex. Set against existing theories for the emplacement of this complex, our investigation failed to find steep outward-dipping fabrics and lineations that would support the emplacement of this ring-complex as a ring-dyke. Instead, we propose that the ring-complex was emplaced as a series of extrusive and intrusive subhorizontal sheets, controlled by a circular zone of deformation, and subsequently domed by the emplacement of the younger central complex. From its gently dipping bulk geometries and a disharmonically folded eutaxitic internal fabric (supported by AMS – anisotropy of magnetic susceptibilty), the earlier rhyolite is reinterpreted as a pyroclastic deposit. The rhyolite was probably deposited against the wall of a subsiding caldera and is now preserved in the SW quadrant of the complex. From primary intrusive contact geometries with pre-Palaeogene country rocks, magnetic fabrics and subtle visible foliations – all of which are gently dipping – the younger and more extensive granitic ring is suggested to have initially been a subhorizontal sheet that is now domed. Only its gently outward-dipping floor is exposed around the ring-complex, and this is for much of its circumference bounded by a circular zone of deformation – a ring-fault. This study highlights the importance of detailed structural investigation in assessing the emplacement of igneous ring-complexes, emphasizing the need to look further than a simple ring-dyke emplacement model.