Pilbarite was described by Simpson (1910) from the Wodgina area of the Pilbara goldfields, Western Australia. The mineral occurs as small nodules enclosed in albite in weathered outcrops of tantalite-rich pegmatites. Occasional residual cores of thorogummite indicate that the pilbarite is pseudomorphous after a primary thorium mineral, probably uranoan thorite. Weathering or hydrothermal alteration of the original thorium mineral yielded what Simpson (1930) considered a chemically related series of distinct species—maitlandite, nicolayite, pilbarite, and hydrothorite. Frondel (1953) has shown that maitlandite, nicolayite, and hydrothorite are minor chemical variants of the phase thorogummite. In a later paper Frondel (1956) mentions pilbarite as an ill-defined substance which needs further study.

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