The industry treats the distributed acoustic sensing (DAS) system, which uses an optical fiber cable in vertical seismic profiling (VSP) data acquisition, as a new and fast-growing technology. The high-quality data set acquired from the DAS acquisition system can produce high-precision VSP images and obtain more detailed checkshots. However, in field data, the acquired VSP data set suffers from strong coherent DAS coupling noise. Many factors may cause coherent DAS coupling noise, such as the cable slapping and ringing due to the physical placement, the regular swing of the wireline in the well, and the uncoupling between the fiber cable and the casing. This DAS coupling noise reduces the signal-to-noise ratio and affects the subsequent processing and interpretation. Removing the DAS coupling noise can help to improve the quality of the VSP data set acquired with the DAS system. We have developed a sparse-optimization-based DAS coupling noise removing method. In the DAS-based VSP data set, the effective signal and the coupling noise have distinct morphological characteristics. The effective VSP signal has a wide bandwidth, whereas the DAS coupling noise appears in some narrow frequency bands in the frequency domain. The continuous wavelet transform and the discrete cosine transform can sparsely represent the effective VSP signal and DAS coupling noise, respectively. Therefore, we choose these two transforms as two sparse dictionaries and combine them to form an overcomplete dictionary. The morphological component analysis (MCA) can use the morphological difference between different components and the overcomplete dictionary to sparsely represent all components in the complicated signal. Based on the MCA theory, we use the block coordinate relaxation algorithm to separate the effective VSP signal and DAS coupling noise. Applications on a synthetic data set and two field data sets have validated the effectiveness of our method.