New Rb–Sr isotopic data from South Portuguese Zone (SPZ) turbidites show that the ⁸⁷Sr/⁸⁶Sr(t) ratio increases from the basal Mértola Formation (Visean–Serpukhovian: 0.706–0.707), through the Mira Formation (Serpukhovian–Bashkirian: 0.706–0.712) to the uppermost Brejeira Formation (Bashkirian–Moscovian: 0.713–0.715). In addition, estimated Nd T_DM model ages for the Mértola (1.29–1.09 Ga), Mira (1.58–1.1 Ga) and Brejeira (1.73–1.37 Ga) formations indicate inverted stratigraphy for their isotopic sources. The isotope geochemical data indicate significant changes in the sources from which the SPZ Carboniferous turbidites are derived, consistent with the progressive denudation of a continental magmatic arc built on the Laurussian margin. Mértola turbidites inherited their geochemical and isotopic characteristics from an adjacent dissected Middle–Late Devonian continental magmatic arc with an intermediate–felsic composition: that is a Laurussian (Rheic magmatic arc)-type source. The progressive erosion of its plutonic roots and older host continental basement rocks are indicated in the Mira and Brejeira formations by the increasing contribution of recycled ancient continental crust. The pronounced similarity between the Nd T_DM model ages and the detrital zircon populations of the Mira and Brejeira formations (SW Iberia) suggest that they share a common Laurussian (West Avalonia/Meguma terrane)-type source but a contribution from Gondwanan (Ossa-Morena)-type sources cannot be discarded.