Abstract We investigate the evolution of the Iberia–Newfoundland margin from Permian post-orogenic extension to Early Cretaceous break-up. We used a Quantitative Basin Analysis approach to integrate seismic stratigraphic interpretations and drill-hole data of two representative sections across the Iberia–Newfoundland margin with kinematic models for lithospheric thinning and subsequent flexural readjustment. We model the distribution of extension and thinning, palaeobathymetry, crustal structure, and subsidence and uplift history as functions of space and time. We start our modelling following post-orogenic extension, magmatic underplating and thermal re-equilibration of the Permian lithosphere. During the Late Triassic–Early Jurassic, broadly distributed, depth-independent lithospheric extension evolved into Late Jurassic–Early Cretaceous depth-dependent thinning as crustal extension progressed from distributed to focused deformation. During this time, palaeobathymetries rapidly deepened across the margin. Modelling of the southern and northern profiles highlighted the rapid development of crustal deformation from south to north over a 5–10 myr period, which accounts for the rapid change in Tithonian–Valanginian, deep- to shallow-water sedimentary facies between the Abyssal Plain and the adjacent Galicia Bank, respectively. Late-stage deformation of both margins was characterized by brittle deformation of the remaining continental crust, which led to exhumation of subcontinental mantle and, eventually, continental break-up and seafloor spreading.

In order to better define the late Eocene clinopyroxene-bearing (cpx) spherule layer and to determine how the ejecta vary with distance from the presumed source crater (Popigai), we searched for the layer at 23 additional sites. We identified the layer at six (maybe seven) of these sites: Deep Sea Drilling Project (DSDP) and Ocean Drilling Program (ODP) Holes 592, 699A, 703A, 709C, 786A, 1090B, and probably 738B. The cpx spherule layer occurs in magnetochron 16n.1n, which indicates an age of ca. 35.4 ± 0.1 Ma for the layer. We found the highest abundance of cpx spherules and associated microtektites in Hole 709C in the northwest Indian Ocean, and we found coesite and shocked quartz in the cpx spherule layer at this site. We also found coesite in the cpx spherule layer at Site 216 in the northeast Indian Ocean. This is the first time that coesite has been found in the cpx spherule layer, and it provides additional support for the impact origin of this layer. In addition, the discovery of coesite and shocked quartz grains (with planar deformation features [PDFs]) supports the conclusion that the pancake-shaped clay spherules associated with quartz grains exhibiting PDFs are diagenetically altered cpx spherules. An Ir anomaly was found associated with the cpx spherule layer at all four of the new sites (699A, 709C, 738B, 1090B) for which we obtained Ir data. The geometric mean of the Ir fluence for the 12 sites with Ir data is 5.7 ng/cm 2 , which is ~10% of the fluence estimated for the Cretaceous-Tertiary boundary. Based on the geographic distribution of the 23 sites now known to contain the cpx spherule layer, and 12 sites where we have good chronostratigraphy but the cpx spherule layer is apparently absent, we propose that the cpx spherule strewn field may have a ray-like distribution pattern. Within one of the rays, the abundance of spherules decreases and the percent microtektites increases with distance from Popigai. Shocked quartz and coesite have been found only in this ray at the two sites that are closest to Popigai. At several sites in the Southern Ocean, an increase in δ 18 O in the bulk carbonate occurs immediately above the cpx spherule layer. This increase may indicate a drop in temperature coincident with the impact that produced the cpx spherule layer.