The Layos Granite forms elongated massifs within the Toledo Complex of central Spain. It is late-tectonic with respect to the F2 regional phase and simultaneous with the metamorphic peak of the region, which reached a maximum temperature of 800–850°C and pressures of 400–600 MPa. Field studies indicate that this intrusion belongs to the “regional migmatite terrane granite” type. This granite is typically interlayered with sill-like veins and elongated bodies of cordierite/garnet-bearing leucogranites. Enclaves are widespread and comprise restitic types (quartz lumps, biotite, cordierite and sillimanite-rich enclaves) and refractory metamorphic country-rocks including orthogneisses, amphibolites, quartzites, conglomerates and calc-silicate rocks. These granites vary from quartz-rich tonalites to melamonzogranites and define a S-type trend on a QAP plot. Cordierite and biotite are the mafic phases of the rocks. The particularly high percentage of cordierite (10%–30%) varies inversely with the silica content. Sillimanite is a common accessory mineral, always included in cordierite, suggesting a restitic origin. The mineral chemistry of the Layos Granite is similar to that of the leucogranites and country-rock peraluminous granulites (kinzigites), indicating a close approach to equilibrium. The uniform composition of plagioclase (An 25 ), the high albitic content of the K-feldspar, the continuous variation in the Fe/Mg ratios of the mafic minerals, and the high Ti content of the biotites (2.5–6.5%) suggest a genetic relationship. Geochemically, the Layos Granite is strongly peraluminous. Normative corundum lies between 4% and 10% and varies inversely with increase in SiO 2 . The CaO content is typically low (<1.25%) and shows little variation; similarly the LILE show a limited range. On many variation diagrams, linear trends from peraluminous granulites to the Layos Granite and associated leucogranite can be observed. The chemical characteristics argue against an igneous fractionation or fusion mechanism for the diversification of the Layos Granite. A restite unmixing model between a granulitic pole (represented by the granulites of the Toledo Complex) and a minimum melt (leucogranites) could explain the main chemical variation of the Layos Granite. Melting of a pelitic protolith under anhydrous conditions (biotite dehydration melting) could lead to minimum-temperature melt compositions and a strongly peraluminous residuum. For the most mafic granites (61–63% SiO 2 ), it is estimated that the trapped restite component must have been around 65%. This high proportion of restite is close to the estimated rheological critical melt fraction, but field evidence suggests that this critical value has been exceeded. This high restite component implies high viscosity of the melt which, together with the anhydrous assemblage of the Layos Granite and the associated leucogranites, indicates H 2 O-undersaturated melting conditions. Under such conditions, the high viscosity magma (crystal-liquid mush) had a restricted movement capacity, leading to the development of parautochthonous plutonic bodies.

Approximately 10–15 vol% of the Neogene Hoyazo dacite consists of Al-rich restite rock inclusions (Al 2 O 3 = 20–45%) and monocrystal inclusions derived therefrom. Restite material and dacitic melt were formed syngenetically from a (semi-)pelitic rock sequence by means of anatexis. Restite rock fragments and dacite show similar high δ 18 O values (13–16‰) corresponding to those found for sedimentary material. Striking monocrystal restite inclusions in the dacite rock are graphite crystals measuring a few hundred μm, 0.5–10 mm blue cordierite crystals and 2–10 mm ruby red crystals of almandine-rich garnet (1.1 ±0.2 vol%). Although the almandine crystals are perfectly euhedral, they are identical in every respect to the crystals found in the Al-rich restite rock inclusions and cannot be crystallisation products of the magmatic melt. The dacite also contains many inclusions of quartz gabbroic and basaltoid material which contains inclusions identical to the restite material found in the dacitic glass base. Many basaltoid inclusions show well-developed chilled borders. These inclusions may represent a more mafic magma of deeper origin which mixed with some dacite magma before mingling into it.

The thermodynamic relations embodied in the Quasicrystalline Model of Burnham and Nekvasil (1986), as recently extended by the author, have been used to quantitatively assess the feldspar-quartz liquidus relations in two I-type (Jindabyne and Moruya) and two S-type (Bullenbalong and Dalgety) suites of Australian granites, using analytical data provided by B. W. Chappell and co-workers. Among the more notable results obtained from these calculations at a constant pressure of 5.0 kbar and X w m = 0.30 (≈2·8wt% H 2 O), for purposes of comparison, are that: (1) felsic melts of remarkably uniform, but distinctive composition can be extracted from each suite, leaving solid residues in amounts up to 65 mol%; (2) all melts from both S-type suites have two feldspars plus quartz on their liquidii, whereas both I-type suites have only plagioclase plus quartz on their liquidii; (3) the total solid residue ranges from 27–63% in the Jindabyne suite, from 15–62% in the Moruya suite, from 30–65% in the Bullenbalong suite, and from 27–65% in the Dalgety suite; (4) liquidus temperatures of the S-type Bullenbalong and Dalgety melts are similar (856° and 860°C), reflecting similar feldspar compositions of An 53 , Or 75 and An 60 , Or 77 , respectively; (5) liquidus temperatures of the I-type Jindabyne and Moruya melts, however, are distinctly different (950° and 894°C), reflecting correspondingly different plagioclase compositions of An 80 , and An 52 ; (6) the calculated liquidus plagioclase composition throughout a given suite is very uniform (±1%) and amounts to as much as 46% of the total rock; and (7) these calculated liquidus and residual plagioclase compositions are also the same, within the uncertainty of measurement, as those of the plagioclase crystal-cores determined optically by A. J. R. White. The only plausible explanation for this remarkable consanguinity in plagioclase liquidus, residue, and crystal-core compositions, hence liquidus temperatures, is that the bulk of the residue is restite, in accordance with the model of White and Chappell (1977). This explanation is corroborated by the very systematic variations in the amounts of individual restite minerals with respect to total restite contents. Accordingly, those members of each suite that contain more than 60% total restite probably closely represent the bulk composition of the source rock, which is dioritic or andesitic for the Jindabyne suite, tonalitic or dacitic for the Moruya suite, pelitic metagreywacke for the Bullenbalong suite, and feldspathic metagreywacke for the Dalgety suite. As a corollary, those members with less than 60% restite must have undergone melt–restite segregation (unmixing), probably during ascent and emplacement.