Synthetic data provided by geoelectric earth models are a powerful tool to evaluate a priori a controlled-source electromagnetic (CSEM) workflow effectiveness. Marlim R3D (MR3D) is an open-source complex and realistic geoelectric model for CSEM simulations of the postsalt turbiditic reservoirs at the Brazilian offshore margin. We have developed a 3D CSEM finite-difference time-domain forward study to generate the full-azimuth CSEM data set for the MR3D earth model. To that end, we fabricated a full-azimuth survey with 45 towlines striking the north–south and east–west directions over a total of 500 receivers evenly spaced at 1 km intervals along the rugged seafloor of the MR3D model. To correctly represent the thin, disconnected, and complex geometries of the studied reservoirs, we have built a finely discretized mesh of cells leading to a large mesh with a total of approximately 90 million cells. We computed the six electromagnetic field components (Ex, Ey, Ez, Hx, Hy, and Hz) at six frequencies in the range of 0.125–1.25 Hz. In our efforts to mimic noise in real CSEM data, we summed to the data a multiplicative noise with a 1% standard deviation. Both CSEM data sets (noise free and noise added), with inline and broadside geometries, are distributed for research or commercial use, under the Creative Common License, at the Zenodo platform.