Lasnierite, (Ca,Sr)(Mg,Fe)2Al(PO4)3, is a new phosphate mineral from Mt. Ibity, close to Itremo, central Madagascar. The mineral was found as inclusions accompanying blue lazulite and many other minerals in blue metaquartzite occasionally used as a gemstone or ornamental stone. The crystals were very small and embedded in quartz so that they could not be extracted mechanically, precluding any “classical” X-ray diffraction on either single-crystal or powder sample. Hence, Focused Ion Beam (FIB) lamellae were extracted and the structure was successfully solved and refined using the recently proposed method of precession electron diffraction tomography (PEDT) associated to dynamical refinement. This underlines the efficiency of this new method for defining mineral species on volumes too small to be manipulated by classical means of X-ray diffraction. Accompanying minerals include various phosphates, sulfates, oxides and silicates. Lasnierite occurs as transparent, near-colourless bladed crystals up to 120 × 60 μm in section. Only five crystals have been identified yet in our samples. The empirical formula, based on wavelength dispersive spectrometry (WDS) electron microprobe analyses and calculated on 12 (O+F) atoms per formula unit, is (Ca0.59Sr0.37)∑0.96(Mg1.42Fe0.54)∑1.96Al0.87(P2.99Si0.01)∑3.00(O11.41F0.59)∑12. LA-ICPMS shows that concentrations of Li, Be and B are below the detection limit. The calculated density based on the empirical formula is 3.162 g cm−3. Lasnierite is orthorhombic, space group Pbcn, with unit-cell parameters: a = 6.2771(3) Å, b = 17.684(3) Å, c = 8.1631(4) Å, Z = 4 and V = 906.1(2) Å3. The structure is new. The Raman spectra show characteristic peaks at 99, 122, 278, 418, 510, 569, 590, 621, 661, 985, 1028, 1040, 1063, 1100, 1126 and 1148 cm−1 (most intense bands are italicised). Raman spectra also show the absence of H2O and CO2.
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Research Article|
March 01, 2019
Lasnierite, (Ca,Sr)(Mg,Fe)2Al(PO4)3, a new phosphate accompanying lazulite from Mt. Ibity, Madagascar: an example of structural characterization from dynamical refinement of precession electron diffraction data on submicrometre sample
Benjamin Rondeau;
1
Laboratoire de Planétologie et Géodynamique, CNRS, UMR 6112, Université de Nantes
, 2 rue de la Houssinière, BP 92208, 44322Nantes cedex 3, France
Corresponding author, e-mail: [email protected]
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Bertrand Devouard;
Bertrand Devouard
2
Aix-Marseille Université, CNRS, INRA, IRD, Coll France, CEREGE UM34
, 13545Aix en Provence, France
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Damien Jacob;
Damien Jacob
3
Unité Matériaux et Transformations, CNRS, UMR 8207, Université de Lille
, 59655Villeneuve d’Ascq, France
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Pascal Roussel;
Pascal Roussel
4
Unité de Catalyse et Chimie du Solide, CNRS, UMR 8181, Université de Lille
, 59655Villeneuve d’Ascq, France
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Nicolas Stephant;
Nicolas Stephant
5
Institut des Matériaux Jean Rouxel, CNRS-UMR 6502, Université de Nantes
, 2 rue de la Houssinière, BP32229, 44322Nantes cedex 3, France
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Constance Boulet;
Constance Boulet
1
Laboratoire de Planétologie et Géodynamique, CNRS, UMR 6112, Université de Nantes
, 2 rue de la Houssinière, BP 92208, 44322Nantes cedex 3, France
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Valentin Mollé;
Valentin Mollé
1
Laboratoire de Planétologie et Géodynamique, CNRS, UMR 6112, Université de Nantes
, 2 rue de la Houssinière, BP 92208, 44322Nantes cedex 3, France
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Marianna Corre;
Marianna Corre
1
Laboratoire de Planétologie et Géodynamique, CNRS, UMR 6112, Université de Nantes
, 2 rue de la Houssinière, BP 92208, 44322Nantes cedex 3, France
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Emmanuel Fritsch;
Emmanuel Fritsch
5
Institut des Matériaux Jean Rouxel, CNRS-UMR 6502, Université de Nantes
, 2 rue de la Houssinière, BP32229, 44322Nantes cedex 3, France
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Cristiano Ferraris;
Cristiano Ferraris
6
Laboratoire de Physique des Milieux Condensés, CNRS, UMR 7590, Muséum National d’Histoire Naturelle
, 61 rue Buffon, 75005Paris, France
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Gian Carlo Parodi
Gian Carlo Parodi
6
Laboratoire de Physique des Milieux Condensés, CNRS, UMR 7590, Muséum National d’Histoire Naturelle
, 61 rue Buffon, 75005Paris, France
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1
Laboratoire de Planétologie et Géodynamique, CNRS, UMR 6112, Université de Nantes
, 2 rue de la Houssinière, BP 92208, 44322Nantes cedex 3, France
Bertrand Devouard
2
Aix-Marseille Université, CNRS, INRA, IRD, Coll France, CEREGE UM34
, 13545Aix en Provence, France
Damien Jacob
3
Unité Matériaux et Transformations, CNRS, UMR 8207, Université de Lille
, 59655Villeneuve d’Ascq, France
Pascal Roussel
4
Unité de Catalyse et Chimie du Solide, CNRS, UMR 8181, Université de Lille
, 59655Villeneuve d’Ascq, France
Nicolas Stephant
5
Institut des Matériaux Jean Rouxel, CNRS-UMR 6502, Université de Nantes
, 2 rue de la Houssinière, BP32229, 44322Nantes cedex 3, France
Constance Boulet
1
Laboratoire de Planétologie et Géodynamique, CNRS, UMR 6112, Université de Nantes
, 2 rue de la Houssinière, BP 92208, 44322Nantes cedex 3, France
Valentin Mollé
1
Laboratoire de Planétologie et Géodynamique, CNRS, UMR 6112, Université de Nantes
, 2 rue de la Houssinière, BP 92208, 44322Nantes cedex 3, France
Marianna Corre
1
Laboratoire de Planétologie et Géodynamique, CNRS, UMR 6112, Université de Nantes
, 2 rue de la Houssinière, BP 92208, 44322Nantes cedex 3, France
Emmanuel Fritsch
5
Institut des Matériaux Jean Rouxel, CNRS-UMR 6502, Université de Nantes
, 2 rue de la Houssinière, BP32229, 44322Nantes cedex 3, France
Cristiano Ferraris
6
Laboratoire de Physique des Milieux Condensés, CNRS, UMR 7590, Muséum National d’Histoire Naturelle
, 61 rue Buffon, 75005Paris, France
Gian Carlo Parodi
6
Laboratoire de Physique des Milieux Condensés, CNRS, UMR 7590, Muséum National d’Histoire Naturelle
, 61 rue Buffon, 75005Paris, France
Corresponding author, e-mail: [email protected]
Publisher: Deutsche Mineralogische Gesellschaft, Sociedad Española de Mineralogia, Societá Italiana di Mineralogia e Petrologia, Société Francaise de Minéralogie
Received:
05 Jul 2018
Revision Received:
11 Oct 2018
Accepted:
11 Oct 2018
First Online:
14 May 2019
Online ISSN: 1617-4011
Print ISSN: 0935-1221
© 2019 E. Schweizerbart’sche Verlagsbuchhandlung, 70176 Stuttgart, Germany
European Journal of Mineralogy (2019) 31 (2): 379–388.
Article history
Received:
05 Jul 2018
Revision Received:
11 Oct 2018
Accepted:
11 Oct 2018
First Online:
14 May 2019
Citation
Benjamin Rondeau, Bertrand Devouard, Damien Jacob, Pascal Roussel, Nicolas Stephant, Constance Boulet, Valentin Mollé, Marianna Corre, Emmanuel Fritsch, Cristiano Ferraris, Gian Carlo Parodi; Lasnierite, (Ca,Sr)(Mg,Fe)2Al(PO4)3, a new phosphate accompanying lazulite from Mt. Ibity, Madagascar: an example of structural characterization from dynamical refinement of precession electron diffraction data on submicrometre sample. European Journal of Mineralogy 2019;; 31 (2): 379–388. doi: https://doi.org/10.1127/ejm/2019/0031-2817
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Index Terms/Descriptors
- Africa
- cell dimensions
- chemical composition
- color
- crystal structure
- electron diffraction data
- electron probe data
- formula
- gems
- ICP mass spectra
- Indian Ocean Islands
- Madagascar
- mass spectra
- new minerals
- optical properties
- ornamental materials
- phosphates
- physical properties
- Raman spectra
- refinement
- spectra
- X-ray diffraction data
- metaquartzite
- Mount Ibity
- focused ion beam
- precession electron diffraction tomography
- lasnierite
Latitude & Longitude
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